What triggers the bond between Kane and Quinn?

The Moon Goddess declares them fated mates, creating a link that burns with pain when they are apart.

Why does Quinn give up the Alpha position?

To shield Kane from danger after their fated mate bond is established.

Fated to My Rival Alpha

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Fated to My Rival Alpha — Bitter rivals Kane and Quinn are bound as fated mates by the Moon Goddess and fight to rule their pack together.

Longtime adversaries Kane and Quinn are marked as fated mates by the Moon Goddess, creating a mystical bond that inflicts physical agony whenever they are separated. Quinn surrenders the Alpha title to protect Kane, but pack member Cyrus exposes their connection to the entire group, turning former allies into threats. The pair swear mutual loyalty and set out to claim the crown while abolishing the she-wolf mate law. Their campaign is interrupted when Bloodfang's Varg kidnaps Quinn and reveals he slaughtered Quinn's family. At the Blood Moon ceremony, the two refuse an order to execute each other, instead awakening a shared twin king power that defeats Varg and Cyrus.

Quick answers

What triggers the bond between Kane and Quinn?: The Moon Goddess declares them fated mates, creating a link that burns with pain when they are apart.
Why does Quinn give up the Alpha position?: To shield Kane from danger after their fated mate bond is established.