Why did Valerie leave the palace?

She could no longer endure being a secret lover while Caspian loved her sister Cassia.

What does Caspian do after Valerie leaves?

He realizes he loves Valerie and pursues her to bring her back.

The Alpha King Wants Me Back

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The Alpha King Wants Me Back — A hidden royal lover departs, forcing an alpha king to confront his misplaced devotion.

For five years, Alpha King Caspian of Vetherland maintained Valerie as his concealed companion while his declared affection belonged to her sister, Cassia. The arrangement stripped Valerie of self-worth until she chose to disappear from the palace and build an autonomous life beyond the kingdom's borders. Only in her absence does Caspian recognize that Valerie, not Cassia, holds his true allegiance. He now seeks to reclaim her, yet she has already begun reconstructing her existence on her own terms.

Quick answers

Why did Valerie leave the palace?: She could no longer endure being a secret lover while Caspian loved her sister Cassia.
What does Caspian do after Valerie leaves?: He realizes he loves Valerie and pursues her to bring her back.